Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Kimura, Atsushi
Journal of Nuclear Science and Technology, 60(11), p.1361 - 1371, 2023/11
Times Cited Count:1 Percentile:72.91(Nuclear Science & Technology)The thermal-neutron capture cross section () and resonance integral (I) for Nb among nuclides for decommissioning were measured by an activation method and the half-life of Nb by mass analysis. Niobium-93 samples were irradiated with a hydraulic conveyer installed in the research reactor in Institute for Integral Radiation and Nuclear Science, Kyoto University. Gold-aluminum, cobalt-aluminum alloy wires were used to monitor thermal-neutron fluxes and epi-thermal Westcott's indexes at an irradiation position. A 25-m-thick gadolinium foil was used to sort out reactions ascribe to thermal-and epi-thermal neutrons. Its thickness provided a cut-off energy of 0.133 eV. In order to attenuate radioactivity of Ta due to impurities, the Nb samples were cooled for nearly 2 years. The induced radio activity in the monitors and Nb samples were measured by -ray spectroscopy. In analysis based on Westcott's convention, the and I values were derived as 1.110.04 barn and 10.50.6 barn, respectively. After the -ray measurements, mass analysis was applied to the Nb sample to obtain the reaction rate. By combining data obtained by both -ray spectroscopy and mass analysis, the half-life of Nb was derived as (2.000.15)10 years.
Okita, Shoichiro; Goto, Minoru
Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 10 Pages, 2023/10
Li, C.-Y.; Wang, K.*; Uchibori, Akihiro; Okano, Yasushi; Pellegrini, M.*; Erkan, N.*; Takata, Takashi*; Okamoto, Koji*
Applied Sciences (Internet), 13(13), p.7705_1 - 7705_29, 2023/07
Times Cited Count:1 Percentile:0(Chemistry, Multidisciplinary)Takino, Kazuo; Oki, Shigeo
JAEA-Data/Code 2023-003, 26 Pages, 2023/05
Since next-generation fast reactors aim to achieve a higher core discharge burn-up than conventional reactors do, core neutronics design methods must be refined. Therefore, a suitable analysis condition is required for the analysis of burn-up nuclear characteristics to accomplish sufficient estimation accuracy while maintaining a low computational cost. We investigated the effect of the analysis conditions on the accuracy of estimation of the burn-up nuclear characteristics of next-generation fast reactors in terms of neutron energy groups, neutron transport theory, and spatial mesh. This study treated the following burn-up nuclear characteristics: criticality, burn-up reactivity, control rod worth, breeding ratio, assembly-wise power distribution, maximum linear heat rate, sodium void reactivity, and Doppler coefficient for the equilibrium operation cycle. As a result, it was found that the following conditions were the most suitable: 18-energy-group structure, 6 spatial meshes per assembly with diffusion approximation. Additionally, these conditions should apply to correction factors for energy group structure, spatial mesh and transport effects.
Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Kimura, Atsushi
Journal of Nuclear Science and Technology, 59(11), p.1388 - 1398, 2022/11
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)The present study selected Np among radioactive nuclides and aimed to measure the thermal-neutron capture cross-section for Np in a well-thermalized neutron field by an activation method. A Np standard solution was used for irradiation samples. A thermal-neutron flux at an irradiation position was measured with neutron flux monitors: Sc, Co, Mo, Ta and Au. The Np sample and flux monitors were irradiated together for 30 minutes in the graphite thermal column equipped with the Kyoto University Research Reactor. The similar irradiation was carried out twice. After the irradiations, the Np samples were quantified using 312-keV gamma ray emitted from Pa in a radiation equilibrium with Np. The reaction rates of Np were obtained from gamma-ray peak net counts given by Np, and then the thermal-neutron capture cross-section of Np was found to be 173.84.4 barn by averaging the results obtained by the two irradiations. The present result was in agreement with the reported data given by a time-of-flight method within the limit of uncertainty.
Mineo, Hideaki
Nihon Genshiryoku Gakkai-Shi ATOMO, 64(11), p.617 - 621, 2022/11
In December 2016 Decisions were made by the Government on the Fast Breeder Prototype Reactor "Monju", which were decommissioning of the reactor and installation of a new research reactor at the Monju site. After the decisions, MEXT started research to list reactor candidates suitable for the site. Among the candidates, medium power reactor type of which thermal output less than 10,000 kW was chosen to utilize neutron beams. Then, from 2020, MEXT launched an entrusted business and adopted JAEA, Kyoto University and University of Fukui as the core institutions of the business to carry out the conceptual design. This paper describes the system to proceed the conceptual design and to examine the utilization management of the new research reactor and also shows their status.
Lu, K.; Takamizawa, Hisashi; Katsuyama, Jinya; Li, Y.
International Journal of Pressure Vessels and Piping, 199, p.104706_1 - 104706_13, 2022/10
Times Cited Count:3 Percentile:60.63(Engineering, Multidisciplinary)Ohgama, Kazuya; Takegoshi, Atsushi*; Katagiri, Hiroki; Hazama, Taira
Nuclear Technology, 208(10), p.1619 - 1633, 2022/10
Times Cited Count:3 Percentile:68.71(Nuclear Science & Technology)Nakamura, Shoji; Toh, Yosuke; Kimura, Atsushi; Hatsukawa, Yuichi*; Harada, Hideo
Journal of Nuclear Science and Technology, 59(7), p.851 - 865, 2022/07
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)The present study performed integral experiments of I using a fast-neutron source reactor "YAYOI" of the University of Tokyo to validate evaluated nuclear data libraries. The iodine-129 sample and flux monitors were irradiated by fast neutrons in the Glory hole of the YAYOI reactor. Reaction rates of I were obtained by measurement of decay gamma-rays emitted from I. The validity of the fast-neutron flux spectrum in the Glory hole was confirmed by the ratios of the reaction rates of flux monitors. The experimental reaction rate of I was compared with that calculated with both the fast-neutron flux spectrum and evaluated nuclear data libraries. The present study revealed that the evaluated nuclear data of I cited in JENDL-4.0 should be reduced as much as 18% in neutron energies ranging from 10 keV to 3 MeV, and supported the reported data by Noguere below 100 keV.
Nakamura, Shoji; Endo, Shunsuke; Kimura, Atsushi; Shibahara, Yuji*
KURNS Progress Report 2021, P. 93, 2022/07
In terms of nuclear transmutation studies of minor actinides in nuclear wastes, the present work selected Np among them and aimed to measure the thermal-neutron capture cross-section of Np using a well-thermalized neutron field by a neutron activation method because there have been discrepancies among reported cross-section data. A Np standard solution was used for irradiation samples. The thermal-neutron flux at an irradiation position was measured with flux monitors: Sc, Co, Mo, Ta and Au. The Np sample was irradiated together with the flux monitors for 30 minutes in the graphite thermal column equipped in the Kyoto University Research Reactor. The similar irradiation was repeated once more to confirm the reproducibility of the results. After irradiation, the Np samples were quantified using 312-keV gamma-ray emitted from Pa in radiation equilibrium with Np. The reaction rates of Np were obtained from the peak net counts of gamma-rays emitted from generated Np, and then the thermal-neutron capture cross-section of Np was found to be 173.84.7 barn by averaging the results obtained by the two irradiations. The present result was in agreement with the reported data given by a time-of-flight method within a limit of uncertainty.
Yokoyama, Kenji; Maruyama, Shuhei; Taninaka, Hiroshi; Oki, Shigeo
JAEA-Data/Code 2021-019, 115 Pages, 2022/03
In JAEA, several versions of unified cross-section set for fast reactors have been developed so far; we have developed a new unified cross-section set ADJ2017R, which is an improved version of the unified cross-section setADJ2017 for fast reactors. The unified cross-section set is used for reflecting information of C/E values (analysis / experiment values) obtained by integral experiment analyses in reactor core design via the cross-section adjustment methodology; the values are stored in the standard database for FBR core design. In the methodology, the cross-section set is adjusted by integrating the information such as uncertainty (covariance) of nuclear data, uncertainty of integral experiment / analysis, sensitivity of integral experiment with respect to nuclear data. ADJ2017R basically has the same performance as ADJ2017, but we conducted an additional investigation on ADJ2017 and revised the following two points. The first is to unify the evaluation method of the correlation coefficient of uncertainty caused by experiments (hereinafter referred to as the experimental correlation coefficient). Because it was found that the common uncertainty used in the evaluation of the experimental correlation coefficient was evaluated by two different methods, the experimental correlation coefficients were revised for all experimental data, and the evaluation method was unified. The second is the review of the integral experiment data used for the cross-section adjustment calculation. It was found that one of the experimental values of composition ratio after irradiation of the Am-243 sample has a problem in uncertainty evaluation because its experimental uncertainty is extremely small compared to the others. The cross-section adjustment calculation was, therefore, redone by excluding the experimental value. In the creation of ADJ2017, a total of 719 data sets were analyzed and evaluated, and eventually adopted 620 integral experimental data sets. In contrast, a total of 61
Ohgama, Kazuya; Katagiri, Hiroki; Takegoshi, Atsushi*; Hazama, Taira
Nuclear Technology, 207(12), p.1810 - 1820, 2021/12
Times Cited Count:3 Percentile:45.99(Nuclear Science & Technology)Takezawa, Hiroki*; Tuya, D.; Obara, Toru*
Nuclear Science and Engineering, 195(11), p.1236 - 1246, 2021/11
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)This study introduces new methodologies for integrating fission reactions induced by delayed neutrons into the Multi-Region Integral Kinetic (MIK) code by using a Monte Carlo neutron transport calculation. First, it was confirmed that it is feasible to solve the Integral Kinetic Model (IKM) with delayed neutrons by the forward Euler discretization method in terms of the number of time steps. This can be done with the help of the law of radioactive decay to reflect the delay in the emission of delayed neutrons in the discretized IKM. Second, a new Monte Carlo-based methodology was introduced for calculating the cumulative distribution functions of secondary fission induced by prompt and delayed neutrons. These functions are necessary for the discretized IKM. The results of preliminary verification using the Godiva reactor confirmed the applicability of the new Monte Carlo-based methodology.
Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Kimura, Atsushi
Journal of Nuclear Science and Technology, 58(10), p.1061 - 1070, 2021/10
Times Cited Count:5 Percentile:56.94(Nuclear Science & Technology)In a well-thermalized neutron field, it is principally possible to drive a thermal-neutron capture cross-section without considering an epithermal neutron component. This was demonstrated by a neutron activation method using the graphite thermal column (TC-Pn) of the Kyoto University Research Reactor. First, in order to confirm that the graphite thermal column was a well-thermalized neutron field, neutron irradiation was performed with neutron flux monitors: Au, Co, Sc, Cu, and Mo. The TC-Pn was confirmed to be extremely thermalized on the basis of Westcott's convention, because the thermal-neutron flux component took a constant value regardless of the sensitivity of each flux monitor to epithermal neutrons. Next, as a demonstration, the thermal-neutron capture cross section of Ta(n,)Ta reaction was measured using the graphite thermal column, and then derived to be 20.50.4 barn, which supported the evaluated value of 20.40.3 barn. The Ta nuclide could be useful as a flux monitor that complements the sensitivity between Au and Mo monitors.
Xu, P. G.; Liss, K.-D.*
Quantum Beam Science (Internet), 5(2), p.11_1 - 11_14, 2021/06
Lu, K.; Katsuyama, Jinya; Li, Y.; Yoshimura, Shinobu*
Journal of Pressure Vessel Technology, 143(2), p.021505_1 - 021505_8, 2021/04
Times Cited Count:1 Percentile:10.51(Engineering, Mechanical)Kenzhina, I.*; Ishitsuka, Etsuo; Ho, H. Q.; Sakamoto, Naoki*; Okumura, Keisuke; Takemoto, Noriyuki; Chikhray, Y.*
Fusion Engineering and Design, 164, p.112181_1 - 112181_5, 2021/03
Tritium release into the primary coolant during operation of the JMTR (Japan Materials Testing Reactor) and the JRR-3M (Japan Research Reactor-3M) had been studied. It is found that the recoil release by Li(n,)H reaction, which comes from a chain reaction of beryllium neutron reflectors, is dominant. To prevent tritium recoil release, the surface area of beryllium neutron reflectors needs to be minimum in the core design and/or be shielded with other material. In this paper, as the feasibility study of the tritium recoil barrier for the beryllium neutron reflectors, various materials such as Al, Ti, V, Ni, and Zr were evaluated from the viewpoint of the thickness of barriers, activities after long-term operations, and effects on the reactivities. From the results of evaluations, Al would be a suitable candidate as the tritium recoil barrier for the beryllium neutron reflectors.
Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Kimura, Atsushi
Journal of Nuclear Science and Technology, 58(3), p.259 - 277, 2021/03
Times Cited Count:5 Percentile:53.85(Nuclear Science & Technology)Research and development were made for accuracy improvement of neutron capture cross section data on Am among minor actinides. First, the emission probabilities of decay rays were obtained with high accuracy, and the amount of the ground state of Am produced by reactor neutron irradiation of Am was examined by -ray measurement. Next, the total amount of isomer and ground states was examined by -ray measurement. Thermal-neutron capture cross sections and resonance integrals were derived both for the Am(n,)Am and for Am(n,)Am reactions.
Kenzhina, I.*; Ishitsuka, Etsuo; Okumura, Keisuke; Ho, H. Q.; Takemoto, Noriyuki; Chikhray, Y.*
Journal of Nuclear Science and Technology, 58(1), p.1 - 8, 2021/01
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)The sources and mechanisms for the tritium release into the primary coolant in the JMTR and the JRR-3M containing beryllium reflectors are evaluated. It is found that the recoil release from chain reaction of Be is dominant and its calculation results agree well with trends derived from the measured variation of tritium concentration in the primary coolant. It also indicates that the simple calculation method used in this study for the tritium recoil release from the beryllium reflectors can be utilized for an estimation of the tritium release into the primary coolant for a research and testing reactors containing beryllium reflectors.
Amaya, Masaki; Kakiuchi, Kazuo; Mihara, Takeshi
Proceedings of International Nuclear Fuel Cycle Conference / Light Water Reactor Fuel Performance Conference (Global/Top Fuel 2019) (USB Flash Drive), p.1048 - 1056, 2019/09